The 50 most-cited articles in Journal of the Physical Society of Japan, 2021

Quantum computers can exploit a Hilbert space whose dimension increases exponentially with the number of qubits. In experiment, quantum supremacy has recently been achieved by the Google team by using a noisy intermediate-scale quantum (NISQ) device with over 50 qubits. However, the question of what can be implemented on NISQ devices is still not fully explored, and discovering useful tasks for such devices is a topic of considerable interest. Hybrid quantum-classical algorithms are regarded as well-suited for execution on NISQ devices by combining quantum computers with classical computers, and are expected to be the first useful applications for quantum computing. Meanwhile, mitigation of errors on quantum processors is also crucial to obtain reliable results. In this article, we review the basic results for hybrid quantum-classical algorithms and quantum error mitigation techniques. Since quantum computing with NISQ devices is an actively developing field, we expect this review to be a useful basis for future studies.

Complex oxides with $4d$ and $5d$ transition-metal ions recently emerged as a new paradigm in correlated electron physics, due to the interplay between spin-orbit coupling and electron interactions. For $4d$ and $5d$ ions, the spin-orbit coupling, $ζ$, can be as large as 0.2-0.4 eV, which is comparable with and often exceeds other relevant parameters such as Hund's coupling $J_{\rm H}$, noncubic crystal field splitting $Δ$, and the electron hopping amplitude $t$. This gives rise to a variety of spin-orbit-entangled degrees of freedom and, crucially, non-trivial interactions between them that depend on the $d$-electron configuration, the chemical bonding, and the lattice geometry. Exotic electronic phases often emerge, including spin-orbit assisted Mott insulators, quantum spin liquids, excitonic magnetism, multipolar orderings and correlated topological semimetals. This paper provides a selective overview of some of the most interesting spin-orbit-entangled phases that arise in $4d$ and $5d$ transition-metal compounds.

We theoretically study the stability of magnetic skyrmion crystals (SkXs) in chiral cubic antiferromagnets with the EuPtSi hosting unconventional nanometric SkXs in mind. By performing numerical simulations for a minimal effective spin model with the long-range Dzyaloshinskii-Moriya interaction and the multiple-spin interaction arising from itinerant nature of electrons, we clarify two key ingredients for the emergence of the SkXs in EuPtSi: One is the low-symmetric ordering vectors that lead to the field-direction sensitive SkXs in an external magnetic field, while the other is the synergy between spin-charge and spin-orbit couplings in itinerant magnets that results in the nanometric SkXs. The present study will not only provide the microscopic mechanism of the SkXs in EuPtSi but also guide for a search of further materials hosting short-period SkXs.

Multiple transition phenomena in divalent Eu compound EuAl$_4$ with the tetragonal structure were investigated via the single-crystal time-of-flight neutron Laue technique. At 30.0 K below a charge-density-wave (CDW) transition temperature of $T_{\rm CDW}$ = 140 K, superlattice peaks emerge near nuclear Bragg peaks described by an ordering vector $q_{\rm CDW}$=(0 0 $δ_c$) with $δ_c{\sim}$0.19. In contrast, magnetic peaks appear at $q_2 = (δ_2 δ_2 0)$ with $δ_2$ = 0.085 in a magnetic-ordered phase at 13.5 K below $T_{\rm N1}$ = 15.4 K. By further cooling to below $T_{\rm N3}$ = 12.2 K, the magnetic ordering vector changes into $q_1 = (δ_1 0 0)$ with $δ_1$ = 0.17 at 11.5 K and slightly shifts to $δ_1$ = 0.194 at 4.3 K. No distinct change in the magnetic Bragg peak was detected at $T_{\rm N2}$=13.2 K and $T_{\rm N4}$=10.0 K. The structural modulation below $T_{\rm CDW}$ with $q_{\rm CDW}$ is characterized by the absence of the superlattice peak in the (0 0 $l$) axis. As a similar CDW transition was observed in SrAl$_4$, the structural modulation with $q_{\rm CDW}$ could be mainly…

The presence of different electronic orders other than superconductivity populating the phase diagram of cuprates suggests that they might be the key to disclose the mysteries of this class of materials.In particular charge order in the form of charge density waves (CDW), i.e., the incommensurate modulation of electron density in the CuO2 planes, is ubiquitous across different families and presents a clear interplay with superconductivity.Until recently, CDW had been found to be confined inside a rather small region of the phase diagram, below the pseudogap temperature and the optimal doping.This occurrence might shed doubts on the possibility that such "low temperature phenomenon" actually rules the properties of cuprates either in the normal or in the superconducting states.However, recent resonant X-ray scattering (RXS) experiments are overturning this paradigm.It results that very short-ranged charge modulations permeate a much wider region of the phase diagram, coexisting with CDW at lower temperatures and persisting up to temperatures well above the pseudogap opening.Here we…

We propose a systematic analysis method for identifying essential parameters in various linear and nonlinear response tensors without which they vanish. By using the Keldysh formalism and the Chebyshev polynomial expansion method, the response tensors are decomposed into the model-independent and dependent parts, in which the latter is utilized to extract the essential parameters. An application of the method is demonstrated by analyzing the nonlinear Hall effect in the ferroelectric SnTe monolayer for example. It is shown that in this example the second-neighbor hopping is essential for the nonlinear Hall effect whereas the spin-orbit coupling is unnecessary. Moreover, by analyzing terms contributing to the essential parameters in the lowest order, the appearance of the nonlinear Hall effect can be interpreted by the subsequent two processes: the orbital magneto-current effect and the linear anomalous Hall effect by the induced orbital magnetization. In this way, the present method provides a microscopic picture of responses. By combining with computational analysis, it stimulates…

Shot noise, originating from the discrete nature of electric charge, is generated by scattering processes. Shot-noise measurements have revealed microscopic charge dynamics in various quantum transport phenomena. In particular, beyond the single-particle picture, such measurements have proved to be powerful ways to investigate electron correlation in quantum liquids. Here, we review the recent progress of shot-noise measurements in mesoscopic physics. This review summarizes the basics of shot-noise theory based on the Landauer-Büttiker formalism, measurement techniques used in previous studies, and several recent experiments demonstrating electron scattering processes. We then discuss three different kinds of quantum liquids, namely those formed by, respectively, the Kondo effect, the fractional quantum Hall effect, and superconductivity. Finally, we discuss current noise within the framework of nonequilibrium statistical physics and review related experiments. We hope that this review will convey the significance of shot-noise measurements to a broad range of researchers in…

Conventional spintronics exploit predominately the properties of ferromagnets (FM). The functionalities of the related devices suffer from two detrimental aspects including the stray fields and the gigahertz (GHz) spin dynamics. These intrinsic limits of FMs can be overcome in antiferromagnets (AFMs), resulting from their vanished stray field, and the faster dynamics in the terahertz (THz) range. On the other hand, AFMs are typically inert to the external magnetic fields. A reliable writing, and more importantly, an accurate read-out of these AFM states are often experimentally challenging, which impede their technological applications. By contrast, ferrimagnets (FIMs) exhibit two antiparallel lattices, and the magnetism of these two sublattices can be fully compensated that manifests as AFM-like dynamics. Unlike the weak resistive response of AFMs, the spin transport properties in FIMs is dominated by one particular lattice (or element). One can thus utilize the typical resistive measurements to unambiguously explore the ultrafast spin dynamics of FIMs. Based on the rare-earth iron…

We report the magnetic susceptibility and the magnetization under pressures up to 1.7 GPa above the critical pressure, P c ∼ 1.5 GPa, for H ∥ a, b, and c-axes in the novel spin triplet superconductor UTe 2 .The anisotropic magnetic susceptibility at low pressure with the easy magnetization a-axis changes to the quasi-isotropic behavior at high pressure, revealing a rapid suppression of the susceptibility for a-axis, and a gradual increase of the susceptibility for the b-axis.At 1.7 GPa above P c , magnetic anomalies are detected at T MO ∼ 3 K and T WMO ∼ 10 K.The former anomaly corresponds to long-range magnetic order, most likely antiferromagnetism, while the latter shows a broad anomaly, which is probably due to the development of short range order.The unusual decrease and increase of the susceptibility below T WMO for H ∥ a and b-axes, respectively, indicate the complex magnetic properties at low temperatures above P c .This is related to the interplay between multiple fluctuations dominated by antiferromagnetism, ferromagnetism, valence and Fermi surface instabilities.

We report the magnetoresistance in the novel spin-triplet superconductor UTe2 under pressure close to the critical pressure Pc, where the superconducting phase terminates, for field along the three a, b and c-axes in the orthorhombic structure. The superconducting phase for H // a-axis just below Pc shows a field-reentrant behavior due to the competition with the emergence of magnetic order at low fields. The upper critical field Hc2 for H // c-axis shows a quasi-vertical increase in the H-T phase diagram just below Pc, indicating that superconductivity is reinforced by the strong fluctuations which persist even at high fields above 20T. Increasing pressure leads to the disappearance of superconductivity at zero field with the emergence of magnetic order. Surprisingly, field-induced superconductivity is observed at high fields, where a spin-polarized state is realized due to the suppression of the magnetic ordered phases; the spin-polarized state is favorable for superconductivity, whereas the magnetic ordered phase at low field seems to be unfavorable. The huge Hc2 in the…

In solving optimization problems, objective functions generally need to be minimized or maximized. However, objective functions cannot always be formulated explicitly in a mathematical form for complicated problem settings. Although several regression techniques infer the approximate forms of objective functions, they are at times expensive to evaluate. Optimal points of "black-box" objective functions are computed in such scenarios, while effectively using a small number of clues. Recently, an efficient method by use of inference by sparse prior for a black-box objective function with binary variables has been proposed. In this method, a surrogate model was proposed in the form of a quadratic unconstrained binary optimization (QUBO) problem, and was iteratively solved to obtain the optimal solution of the black-box objective function. In the present study, we employ the D-Wave 2000Q quantum annealer, which can solve QUBO by driving the binary variables by quantum fluctuations. The D-Wave 2000Q quantum annealer does not necessarily output the ground state at the end of the protocol…

In spin caloritronics, a branch of spintronics, the spin degree of freedom is exploited for thermoelectric conversion and thermal transport. Since the inception of spin caloritronics, many experimental and theoretical studies have focused on clarifying the fundamental physics of the heat-to-spin and heat-to-charge current conversion phenomena in magnetic materials and magnetic hybrid structures, such as the spin Seebeck and anomalous Nernst effects. While research on these phenomena is progressing, there are also many spin-caloritronic phenomena that output heat currents. The observations of such phenomena have recently been accomplished through cutting-edge heat detection techniques. The recent developments in spin caloritronics have revealed that the generation, conversion, and transport of heat can be actively controlled by spins and/or magnetism. In this review article, we propose a new concept called spintronic thermal management. With proof-of-concept demonstrations, we introduce the basic principles, behaviors, measurement methods, and heat control functionalities of…

In this review we introduce computer modelling and simulation techniques which are used for ferrimagnetic materials. We focus on models where thermal effects are accounted for, atomistic spin dynamics and finite temperature macrospin approaches. We survey the literature of two of the most commonly modelled ferrimagnets in the field of spintronics--the amorphous alloy GdFeCo and the magnetic insulator yttrium iron garnet. We look at how generic models and material specific models have been applied to predict and understand spintronic experiments, focusing on the fields of ultrafast magnetisation dynamics, spincaloritronics and magnetic textures dynamics and give an outlook for modelling in ferrimagnetic spintronics.

We report the inelastic X-ray scattering (IXS) experimental results of iridium oxide Ca5Ir3O12 with a strong spin–orbit interaction, showing the hidden order at 105 K where no superlattice reflections were observed so far. We measured the IXS spectra of Ca5Ir3O12 along Γ–A, Γ–M, Γ–K–M, M–L, and K–H directions in the Brillouin zone of a hexagonal lattice down to 20 K. The obtained phonon spectra show almost no change on cooling; there are no soft phonon modes. However, the superlattice reflections specified by wavevector q=(1/3,1/3,1/3) are observed below 105 K. For the order parameter in the hidden order, the characteristic on intensity for observed superlattice reflections can lead to the irreducible representation A2 order parameter in the point group 31m. Furthermore, the theoretical study indicates that the hidden order at 105 K comes from an electric toroidal dipole or higher-order multipole ordering.

Electronic properties of the single crystal of GdV6Sn6, where non-magnetic V-kagome layers are separated by magnetic Gd-triangular lattice, are investigated. GdV6Sn6 exhibits unique magnetotransport properties at low-temperature such as non-linear Hall resistivity and increase of resistance R in magnetic field H as R ~ H^0.75 up to 56 T with Shubnikov-De Haas oscillations. Investigation of the non-magnetic analogue YV6Sn6 and the first principles calculations reveal these properties are relevant to the bands arising from the V-kagome layer. A magnetic transition at 5 K in GdV6Sn6 modifies the transport properties, pointing to a coupling between Gd-spins on the triangular lattice and carriers in the V-kagome layer.

UTe$_2$ is a recently discovered promising candidate for a spin-triplet superconductor. In contrast to conventional spin-singlet superconductivity, spin-triplet superconductivity possesses spin and angular momentum degrees of freedom. To detect these degrees of freedom and obtain the solid evidence of spin-triplet superconductivity in UTe$_2$, we performed $^{125}$Te-NMR measurement. We previously reported that the shoulder signal appears in NMR spectra below the superconducting (SC) transition temperature $T_{\rm c}$ in $H \parallel b$, and that a slight decrease in the Knight shift along the $b$ and $c$ axes ($K_b$ and $K_c$, respectively) below $T_{\rm c}$ at a low magnetic field $H$. To clarify the origin of the shoulder signal and the trace of the decrease in $K_b$, we compared the $^{125}$Te-NMR spectra obtained when $H~\parallel~b$ and $H~\parallel~c$ and measured the $^{125}$Te-NMR spectra for $H~\parallel~b$ up to 14.5~T. The intensity of the shoulder signal observed for $H~\parallel~b$ has a maximum at $\sim 6$~T and vanishes above 10~T, although the superconductivity is…

A polymorph of RuI$_3$ synthesized under high pressure was found to have a two-layered honeycomb structure. The resistivity of RuI$_3$ exhibits a semimetallic behavior, in contrast to insulating properties in $α$-RuCl$_3$. In addition, Pauli paramagnetic behavior was observed in the temperature dependence of a magnetic susceptibility and a nuclear spin-lattice relaxation rate 1/$T_1$. The band structure calculations indicate that contribution of the I 5$p$ components to the low-energy $t_\mathrm{2g}$ bands effectively decreases Coulomb repulsion, leading to semimetallic properties. The physical properties also suggest strong electron correlations in RuI$_3$.

The rare-earth-free ferrimagnet Mn 4 N has attractive features for spintronics applications, because it possesses a perpendicular magnetization, due to a relatively large magnetic anisotropy constant of ~10 5 J m -3 and a small spontaneous magnetization of ~100 kA m -1 , and a large spin polarization (P = 0.8).More crucially, it is possible to reach the magnetic compensation at room temperature, by tuning its constituent element in compounds such as Mn 4-x Ni x N and Mn 4-x Co x N.This is particularly interesting for spin-torque-based spintronics applications, because at the vicinity of the magnetization and/or angular momentum compensation points, the switching currents can be reduced significantly, thereby leading to lower switching energies and higher switching speed.In this review article, we emphasize the importance of epitaxial growth of Mn 4 N films by comparing the results obtained on two different substrates, MgO(001) and SrTiO 3 (001).We then present the achievement of ultrafast current-induced domain wall motion (CIDWM) in Mn 4 N microstrips, and study the magnetic…

In a recent letter [\textit{Phys.~Rev.~Lett.}~\textbf{125}, 085001 (2020)], Dornheim \textit{et al.}~have presented the first \textit{ab initio} path integral Monte Carlo (PIMC) results for the nonlinear electronic density response at warm dense matter (WDM) conditions. In the present work, we extend these considerations by exploring the relation between the nonlinear response and three-/four-body correlation functions from many-body theory. In particular, this connection directly implies a comparably increased sensitivity of the nonlinear response to electronic exchange-correlation (XC) effects, which is indeed confirmed by our analysis over the entire relevant range of densities ($r_s=0.5,\dots,10$) and temperatures ($θ=0.01,\dots,4$). Finally, our work suggests the possibility of deliberately probing the nonlinear regime to experimentally probe three- and potentially even four-body correlation functions in WDM.

We investigate the spin rotational structure of magnetic skyrmions in a tetragonal polar magnet VOSe2O5 via polarized small-angle neutron scattering (SANS). Spin polarization analysis of the scattered neutrons provides consistent evidence for the cycloidal spin modulation in all the incommensurate phases at zero and non-zero magnetic field along the c axis, including the triangular skyrmion-lattice phase. In the vicinity of the skyrmion phase, we performed extensive SANS measurements to unravel a field-induced incommensurate phase (IC-2 state). We discuss the possibility of anisotropic double-q state as an alternative spin structure to provisional square skyrmion-lattice state.

Metamagnetic transitions in the novel spin-triplet superconductor UTe$_2$ were investigated through the newly developed simultaneous measurements of magnetization and sample temperature for the field along the orthorhombic $b$-axis and close to the [011] direction, where reentrant superconductivity (RSC) is detected below and above the first-order metamagnetic transition field $H_{\rm m}$. Combining the Maxwell's relation and the Clausius-Clapeyron equation, we obtained the field dependence of Sommerfeld coefficient $γ$ through the first-order metamagnetic transition. A significant enhancement of the effective mass toward $H_{\rm m}$ were detected for both field directions. On the other hand, above $H_{\rm m}$, the effective mass discontinuously decreases for $H~||~b$, while it discontinuously increases for $H~||~\sim [011]$, which seems to make a crucial role for the RSC.

The excitonic insulator Ta$_2$NiSe$_5$ experiences a first-order structural transition under pressure from rippled to flat layer-structure at Ps = 3 GPa, which drives the system from an almost zero-gap semiconductor to a semimetal. The pressure-induced semimetal, with lowering temperature, experiences a transition to another semimetal with a partial-gap of 0.1-0.2 eV, accompanied with a monoclinic distortion analogous to that occurs at the excitonic transition below Ps. We argue that the partial-gap originates primarily from a symmetry-allowed hybridization of Ta-conduction and Ni-valence bands due to the lattice distortion, indicative of the importance of electron-lattice coupling. The transition is suppressed with increasing pressure to Pc = 8 GPa. Superconductivity with a maximum Tsc = 1.2 K emerges around Pc, likely mediated by strongly electron-coupled soft phonons. The electron-lattice coupling is as important ingredient as the excitonic instability in Ta2NiSe5.

The temperature coefficient α (= dV/dT) of the redox potential (V) in a redox system, or so-called electrochemical Seebeck coefficient, is a key parameter for thermal energy harvesting. We systematically investigated α for Fe2+/Fe3+ in 16 organic solvents, i.e., 8 protic and 8 aprotic solvents. We found that α shows remarkable solvent dependence and is distributed from 0.14 mV/K for glycerin to 3.60 mV/K for acetone. We further found a scaling relation between α and viscosity (η) of the solvent as α ∝ η−0.4. We will discuss solvent dependence of α and the scaling relation in terms of the configuration entropy of the solvent molecules.

We investigate the spin dynamics in the superconducting phase of UTe$_{2}$ by triple-axis inelastic neutron scattering on a single crystal sample. At the wave-vector $\bf{k_1}$=(0, 0.57, 0), where the normal state antiferromagnetic correlations are peaked, a modification of the excitation spectrum is evidenced, on crossing the superconducting transition, with a reduction of the relaxation rate together with the development of an inelastic peak at $Ω$ $\approx$ 1 meV. The low dimensional nature and the the $a$-axis polarization of the fluctuations, that characterise the normal state, are essentially maintained below $T_{sc}$. The high ratio $Ω/k_{B}T_{sc}$ $\approx$ 7.2 contrasts with the most common behaviour in heavy fermion superconductors.

In linear control systems, a feedback loop is often adopted, but this limits the bandwidth of the controlled system. Moreover, owing to the presence of noise in the feedback, which is essentially linked to the measurement of the fed-back variables, the bandwidth is reduced in order to maintain the desired performance. This short note proposes the utilization of the concept of stochastic resonance to overcome this limitation. A simple, but effective, nonlinearity is introduced in the controller leading to improved performances in terms of signal-to-noise ratio when dealing with tracking of small-amplitude signals.

Spin waves and their quanta magnons are collective excitation of electron spins in magnetic materials which can serve as information carriers for future low-power-consumption computing systems. Ferrimagnetic thin-film iron garnets are considered as an ideal platform for spin waves due to the low Gilbert damping. Here, we review the recent progress of magnonics based on thin-film iron garnets, including the yttrium iron garnet (YIG). Short-wavelength spin waves with dispersion relation governed by the exchange interaction have recently been reported in low damping YIG thin films. Periodical nanostructure thin-film iron garnets enrich the functionalities of magnonic crystals. In addition, pure spin currents in adjacent heavy metal layers could induce magnetic auto-oscillations and propagating spin waves in thin-film iron garnets. The broken inversion symmetry has also been found in thin-film iron garnets probed by chiral spin-wave group velocities. We conclude that thin-film iron garnets hold a bright future for magnon based logic devices and circuits.

We have theoretically investigated thermoelectric (TE) effects of narrow-gap single-walled carbon nanotubes (SWCNTs) with randomly substituted nitrogen (N) impurities, i.e., N-substituted (20,0) SWCNTs with a band gap of 0.497 eV. For such a narrow-gap system, the thermal excitation from the valence band to the conduction band contributes to its TE properties even at the room temperature. In this study, the N-impurity bands are treated with both conduction and valence bands taken into account self-consistently. We found the optimal N concentration per unit cell, $c_{\rm opt}$, which gives the maximum power factor ($PF$) for various temperatures, e.g., $PF=$0.30$\rm{W/K^2m}$ with $c_{\rm opt}=3.1\times 10^{-5}$ at 300K. In addition, the electronic thermal conductivity has been estimated, which turn out to be much smaller than the phonon thermal conductivity, leading to the figure of merit as $ZT\sim 0.1$ for N-substituted (20,0) SWCNTs with $c_{\rm opt}=3.1\times 10^{-5}$ at 300K.

The research into insulating ferrimagnetic garnets has gained enormous momentum in the past decade.This is partly due to the improvement in the techniques to grow high-quality ultrathin films with desirable properties and the advances in understanding the spin transport within the ferrimagnetic garnets and through their interfaces with conducting materials.In recent years, we have seen remarkable progress in controlling the magnetization state of ferrimagnetic garnets by electrical means in suitable heterostructures and device architectures.These advances have readily placed ferrimagnetic garnets in a favorable position for the future development of insulating spintronic concepts.The purpose of this article is to review recent experimental results of the current-induced magnetization control and associated phenomena in ferrimagnetic garnets, as well as to discuss future directions in this rapidly evolving area of spintronics.

NaAlSi is an sp electron superconductor crystallizing in a layered structure of the anti-PbFCl type with a relatively high transition temperature Tc of ~7 K. Recent electronic state calculations revealed the presence of topological nodal lines in the semimetallic band structure, which attracted much attention owing to the superconductivity. However, experimental investigation remained limited because of the lack of single crystals. Here, we successfully prepared single crystals of NaAlSi by a Na-Ga flux method and characterized their superconducting and normal-state properties through electrical resistivity, magnetization, and heat capacity measurements. A sharp superconducting transition with a Tc of 6.8 K is clearly observed, and heat capacity data suggest an anisotropic superconducting gap. Surprisingly, despite the sp electron system, the normal state is governed by the electron correlations, which is indicated by a T2 resistivity and a Wilson ratio of 2.0. The origin of the electron correlation may be related to the orthogonal saddle-shaped Fermi surfaces derived from the Si px…

We have measured thermoelectric properties of Ta2PdX6 (X=S, Se) around room temperature using single crystal samples. We find that the power factor of Ta2PdX6 is relatively high from middle-low to room temperatures, and notably Ta2PdSe6 shows the largest power factor among thermoelectric materials with an electrical conductivity of 10-2 Ωcm at 300 K. Ta2PdS6 will be a possible candidate for a Peltier cooling material if the lattice thermal conductivity is reduced by chemical substitution.

Superconductivity in layered cuprates is induced by doping holes into a parent antiferromagnetic insulator. It is now recognized that another common emergent order involves charge stripes, and our understanding of the relationship between charge stripes and superconductivity has been evolving. Here we review studies of 214 cuprate families obtained by doping La$_2$CuO$_4$. Charge-stripe order tends to compete with bulk superconductivity; nevertheless, there is plentiful evidence that it coexists with two-dimensional superconductivity. This has been interpreted in terms of pair-density-wave superconductivity, and the perspective has shifted from competing to intertwined orders. In fact, a new picture of superconductivity based on pairing within charge stripes has been proposed, as we discuss.

The presence of charge order in high-transition-temperature copper oxides (high-Tc cuprates) was identified a decade ago. Now it is a universally observed order like the antiferromagnetic and the superconducting orders of the cuprates. The charge order shows up in various forms depending on materials, and it overlaps other orders in the phase diagram. Because of this diversity and complexity it has been far from clear whether or not the charge order has a direct relevance to superconductivity and to the mysterious pseudogap phenomenon. However, the research development in the last few years has been successful in revealing universal aspects of the charge order and its fluctuations. It turns out that the charge order is compatible with superconductivity, and that its fluctuations have high onset temperature and high energy scale comparable to those of the pseudogap. The charge order correlations might be indispensable for creating the pseudogap and possibly generating high-Tc superconductivity by collaborating with spin and pairing correlations.

We performed $^{59}$Co nuclear magnetic and quadrupole resonance (NMR and NQR) measurements under pressure on a single-crystalline CeCoSi, which undergoes an unresolved phase transition at $T_0$. The NQR spectra clearly showed that the phase transition at $T_0$ is nonmagnetic, but any symmetry lowering at the Co site was not seen irrespective of the feature of second-order phase transition. By contrast, the NMR spectra were split by the induced magnetic field perpendicular to the external magnetic field. These results show that the phase below $T_0$ is not a simple paramagnetic state but is most likely electric multipolar ordered state of Ce $4f$ electrons. The development of the Kondo effect by applying pressure is thought to be crucial to stabilize this state and to show novel features beyond commonality of tetragonal Ce-based systems.

We performed 121/123Sb-nuclear quadrupole resonance (NQR) measurements on the superconducting (SC) line-nodal material CaSb2 in order to investigate electronic properties in the normal and SC states from a microscopic point of view. In the normal state, the nuclear spin-lattice relaxation rate 1/T1 for the Sb(1) site, which is responsible for the line-nodal parts, is approximately proportional to temperature, indicating the conventional Fermi liquid state. From comparison with band structure calculations, it is considered that the NQR properties related to the line-nodal character are hidden because the conventional behavior originating from Fermi-surface parts away from the nodes is dominant. In the SC state, a clear coherence peak just below the transition temperature and an exponential decrease at lower temperatures were observed in 1/T1. These results strongly suggest that conventional s-wave superconductivity with a full gap is realized in CaSb2.

We report on the superconductivity in ternary transition metal tellurides Ta2Pd3Te5 and Nb2Pd3Te5, which have a one-dimensional crystal structure. Single-crystalline and polycrystalline samples of Ta2Pd3Te5 show nonmetallic electron conduction, while Ti or W doping results in metallic behavior with a bulk superconducting transition at 2-4 K. In contrast, the polycrystalline samples of Nb2Pd3Te5, which are found to be isostructural to Ta2Pd3Te5, show a bulk superconducting transition at 3.3 K. The crystal structure and physical properties of Ta2Pd3Te5 and Nb2Pd3Te5 are also discussed in comparison with a candidate excitonic insulator Ta2NiSe5.

We theoretically study electric quadrupole orders in f-electron systems on the fcc lattice. Qudrupole degrees of freedom $O_{20}$ and $O_{22}$ originate in the non-Kramers doublet ground state $Γ_3$ of ion with $f^2$ electron configuration. For discussing quadrupole orders, we use a minimal model with isotropic ($J$) and anisotropic ($K$) nearest-neighbor interactions, and determine the phase diagram using a four-site mean-field approximation at zero and finite temperatures. Quadrupoles couple the $Γ_3$ doublet to the singlet excited state $Γ_1$, and its effects on canting antiferro orders are examined in detail. We found that this coupling leads to a rich phase diagram including two- and four-sublattice antiferro phases, and that two phases show a partial order of quadrupoles at finite temperatures.

The variational principle of the Onsager-Machlup integral is used to describe the stochastic dynamics of a micromachine, such as an enzyme, characterized by odd elasticity. The obtained most probable path is found to become non-reciprocal in the presence of odd elasticity and is further related to the entropy production.

Studies on the interplay between the charge order and the $d$-wave superconductivity in the copper-oxide high $T_{\rm c}$ superconductors are reviewed with a special emphasis on the exploration based on the unconventional concept of the electron fractionalization and its consequences supported by solutions of high-accuracy quantum many-body solvers. Severe competitions between the superconducting states and the charge inhomogeneity including the charge/spin striped states revealed by the quantum many-body solvers are first addressed for the Hubbard models and then for the {\it ab initio} Hamiltonians of the cuprates derived without adjustable parameters to represent the low-energy physics of the cuprates. The charge inhomogeneity and superconductivity are born out of the same mother, namely, the carrier attraction arising from the strong Coulomb repulsion near the Mott insulator (Mottness) and accompanied electron fractionalization. The same mother makes the severe competition of the two brothers inevitable. The electron fractionalization has a remarkable consequences on the…

We investigate the presence of an acoustic-quasi-elastic interaction contribution in the IXS spectra of liquid water at 301K using inelastic x-ray scattering with sub-meV energy resolution at momentum transfers 0.77<=Q<=4.20 /nm. The contribution appears due to the overlap the acoustic mode with the tail the quasi-elastic mode and is fully consistent with hydrodynamic theory. Incorporating this interaction allows us to describe the dynamic structure factor, S(Q,w), without introducing an extra mode, and may help explain earlier contradictory interpretations. The sound velocity, and relative intensity of the quasi-elastic and acoustic mode, plateau for Q>2/nm at values consistent with a viscoelastic generalization of the Landau-Placzek relation.

We propose a model for a thermally driven microswimmer in which three spheres are connected by two springs with odd elasticity. We demonstrate that the presence of odd elasticity leads to the directional locomotion of the stochastic microswimmer.

This paper reports a novel method for supervised machine learning based on the mathematical formalism that supports quantum mechanics. The method uses projective quantum measurement as a way of building a prediction function. Specifically, the relationship between input and output variables is represented as the state of a bipartite quantum system. The state is estimated from training samples through an averaging process that produces a density matrix. Prediction of the label for a new sample is made by performing a projective measurement on the bipartite system with an operator, prepared from the new input sample, and applying a partial trace to obtain the state of the subsystem representing the output. The method can be seen as a generalization of Bayesian inference classification and as a type of kernel-based learning method. One remarkable characteristic of the method is that it does not require learning any parameters through optimization. We illustrate the method with different 2-D classification benchmark problems and different quantum information encodings.

The transport and thermodynamic properties of $β$-ReO$_{2}$ crystallizing in a nonsymmorphic structure were studied using high-quality single crystals. An extremely large magnetoresistance (XMR) reaching 22,000 $\%$ in a transverse magnetic field of 10 T at 2 K was observed. However, distinguished from other topological semimetals with low carrier densities that show XMR, $β$-ReO$_{2}$ has a high electron carrier density of 1 $\times$ $10^{22}$ cm$^{-3}$ as determined by Hall measurements and large Fermi surfaces in the electronic structure. In addition, a small Fermi surface with a small effective mass was evidenced by de Haas-van Alphen oscillation measurements. The previous band structure calculations [S. S. Wang, et al., Nat. Commun. 8, 1844 (2017)] showed that two kinds of loops made of Dirac points of hourglass-shaped dispersions exist and are connected to each other by a point to form a string of alternating loops, called the Dirac loop chain (DLC), which are protected by the multiple glide symmetries. Our first-principles calculations revealed the complex Fermi surfaces with…

Magnetic skyrmions, which are topologically protected particle-like spin textures, exhibit Brownian motion at ambient temperatures in a ferromagnetic thin film. The potential applications of a skyrmions’ diffusive motion to the ultra-low energy stochastic and Brownian computation make research on its thermal dynamics necessary. Herein we experimentally demonstrate the mobility anomaly of the diffusion coefficients in one-dimensional diffusion processes. In addition, we observed a chiral property in the velocity–position correlation functions. The results are discussed in the context of Brownian motion in the shallow potential fluctuations. The data indicate the importance of the chiral property of skyrmions in Brownian motion.

Ultrafast control of thin film nanomagnets using femtosecond laser pulses has attracted considerable attention for future ultrafast and energy-efficient photo-spintronics storage=memory devices.Single femtosecond laser pulse magnetization switching without an applied external magnetic field has been recently observed on various metallic thin films.Herein, a recent understanding of the physical mechanism behind single-shot all-optical magnetization switching and perspectives are described.

We analysed the generalisation performance of a binary perceptron with quantum fluctuations using the replica method. An exponential number of local minima dominate the energy landscape of the binary perceptron. Local search algorithms often fail to identify the ground state of a binary perceptron. In this study, we considered the teacher-student learning method and computed the generalisation error of a binary perceptron with quantum fluctuations. Due to the quantum fluctuations, we can efficiently find robust solutions that have better generalisation performance than the classical model. We validated our theoretical results through quantum Monte Carlo simulations. We adopted the replica symmetry (RS) ansatz assumption and static approximation. The RS solutions are consistent with our simulation results, except for the relatively low strength of the transverse field and high pattern ratio. These deviations are caused by the violation of ergodicity and static approximation. After accounting for the deviation between the RS solutions and numerical results, the enhancement of…

The pressure-induced insulator to metal transition (IMT) of layered magnetic nickel phosphorous tri-sulfide NiPS 3 was studied in-situ under quasi-uniaxial conditions by means of electrical resistance (R) and X-ray diffraction (XRD) measurements.This sluggish transition is shown to occur at 35 GPa.Transport measurements show no evidence of superconductivity to the lowest measured temperature (∼2 K).The structure results presented here differ from earlier insitu work that subjected the sample to a different pressure state, suggesting that in NiPS 3 the phase stability fields are highly dependent on strain.It is suggested that careful control of the strain is essential when studying the electronic and magnetic properties of layered van der Waals solids.

In this study, we measure the magnetic field and temperature variations of the magnetization \(M(H,T)\) of the cubic chiral compound EuPtSi and extensively investigate the magnetic phase transitions in a wide temperature range down to 60 mK. The incommensurate–commensurate transition at \(T_{\text{N}}^{*} \simeq 2.5\) K in the helical state, which has not been observed in transport or thermodynamic measurements, is exclusively detected in M(T) for H || 〈111〉. \(T_{\text{N}}^{*}\) shows a rapid decrease in H. For H || [100] and [111], M(H) at T < 100 mK showed that the helical q vectors are depinned from the preferred orientations at \(H \gtrsim 10\) kOe and gradually rotate toward the field directions as H increases. The skyrmion lattice phase (A-phase) field-induced in H || 〈111〉 only above 0.4 K in equilibrium conditions can be created at 60 mK under field cooling, with a sharp tilted plateau structure developing in M(H) of the A-phase. A similar metastable state is also created below 100 mK for the A′ phase induced by H || 〈100〉 at \(T \gtrsim 0.3\) K in equilibrium conditions.…

On the basis of the point charge model, we formulate the crystalline electronic field (CEF) Hamiltonian $H_{\rm CEF}$ in the rare-earth based quasicrystal (QC) and approximant crystal (AC) with ligand ions located at pseudo 5-fold configurations by using the operator equivalent method. By setting the total angular momentum $J=7/2$, the CEF in the quantum critical QC Au$_{51}$Al$_{34}$Yb$_{15}$ and the 1/1 AC Au$_{51}$Al$_{35}$Yb$_{14}$ is analyzed with consideration for the effect of Al/Au mixed sites. We find that the ratio of the valences of ligand ions $x=Z_{\rm Al}/Z_{\rm Au}$ plays an important role in characterizing the CEF ground state. As $x$ decreases from $x=3$, the 4f wave function of the CEF ground state with the flat shape lying in the mirror plane is deformed around $x\approx 0.8$ to the flat shape perpendicular to the pseudo 5-fold axis at $x=0$. The formulated $H_{\rm CEF}$ by $J$ is generally applicable to rare-earth-based QCs and ACs, which is useful to analyze the CEF.

The aggregation behavior of cavitation bubbles in liquids has vital effect on the ultrasonic cavitation effect. The secondary Bjerknes force between two bubbles is one of the mechanisms underlying this aggregation behavior of bubbles. In this paper, the secondary Bjerknes force between two bubbles, which are irradiated by a high-intensity ultrasonic field (near the Blake threshold), is numerically calculated. In addition, the influences of pressure amplitude, physical parameters, distance between the bubbles and equilibrium radii of bubble-pairs on the secondary Bjerknes force are also investigated. The results show that when the pressure amplitude is greater than Blake threshold, the secondary Bjerknes force between bubbles of equal and unequal equilibrium radii increases markedly with pressure amplitude increasing. The secondary Bjerknes force decreases with the increase of liquid viscosity, surface tension and density, while increases with the saturated vapor pressure increasing. For the two bubbles of larger equilibrium radii, the distance between two bubbles has an obvious…

We study a topological physics in a one-dimensional nonlinear system by taking an instance of a mechanical rotator model with alternating spring constants. This nonlinear model is smoothly connected to an acoustic model described by the Su-Schrieffer-Heeger model in the linear limit. We numerically show that quench dynamics of the kinetic and potential energies for the nonlinear model is well understood in terms of the topological and trivial phases defined in the associated linearized model. It indicates phenomenologically the emergence of the edge state in the topological phase even for the nonlinear system, which may be the bulk-edge correspondence in nonlinear system.